Influence of multi-walled carbon nanotubes on electrochemical performance of transparent graphene electrodes

Ki Seok Kim, Kyong Yop Rhee, Soo Jin Park

Research output: Contribution to journalArticlepeer-review

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Abstract

In this work, carbon-carbon nanocomposites as transparent electrodes were prepared by a chemical reduction of graphite oxide (GO) and multi-walled carbon nanotubes (MWNTs). The electric, optical, and electrochemical properties of graphene-MWNT nanocomposites (G-MCs) were investigated as a function of the MWNT content. It was found that chemically bonded G-MCs were successfully formed with a reduction of the functional groups of the GO and acid-treated MWNTs, resulting in the conjugation of 1D MWNTs onto a 2D graphene surface. The electrical conductivity of the graphene was significantly enhanced by introducing the MWNTs. In addition, the G-MCs showed improved current density and high efficiency compared with graphene alone. This indicated that the improved electrochemical performance of the G-MCs can be attributed to the increase in the activity and electrical conductivity enhanced by π-π interaction between graphene and MWNTs.

Original languageEnglish
Pages (from-to)1301-1306
Number of pages6
JournalMaterials Research Bulletin
Volume46
Issue number8
DOIs
StatePublished - Aug 2011

Bibliographical note

Funding Information:
This work was supported by the Material Source Technology Development Business of the Ministry of Knowledge Economy, Korea .

Keywords

  • A. Interfaces
  • A. Nanostructures
  • D. Electrical properties
  • D. Electrochemical properties
  • D. Optical properties

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