TY - JOUR
T1 - Conceptual Design of a Fischer-Tropsch Reactor in a Gas-to-Liquid Process
AU - Lee, Hyun Jung
AU - Choi, Ju Hwan
AU - Garforth, Arthur
AU - Hwang, Sungwon
N1 - Publisher Copyright:
© 2015 American Chemical Society.
PY - 2015/7/8
Y1 - 2015/7/8
N2 - This research focused on the design and optimization of a two-phase Fischer-Tropsch (F-T) reactor in a gas-to-liquid (GTL) process. For the design of the F-T reactor, the overall process configuration was developed using Aspen HYSYS software. Various reaction mechanisms for the F-T process over iron-based catalysts were reviewed from the published literature. The F-T kinetics was adopted for reactor modeling, and the reaction kinetic parameters were adjusted to increase the accuracy of the modeling results. Furthermore, the effects of catalyst size, catalyst active sites, and reactor configuration were embedded into the modeling. The yields of the F-T process were analyzed under various operating conditions. Finally, operating conditions, such as the temperature and pressure of the two-phase-reactor model, were optimized to maximize the yield of hydrocarbon products.
AB - This research focused on the design and optimization of a two-phase Fischer-Tropsch (F-T) reactor in a gas-to-liquid (GTL) process. For the design of the F-T reactor, the overall process configuration was developed using Aspen HYSYS software. Various reaction mechanisms for the F-T process over iron-based catalysts were reviewed from the published literature. The F-T kinetics was adopted for reactor modeling, and the reaction kinetic parameters were adjusted to increase the accuracy of the modeling results. Furthermore, the effects of catalyst size, catalyst active sites, and reactor configuration were embedded into the modeling. The yields of the F-T process were analyzed under various operating conditions. Finally, operating conditions, such as the temperature and pressure of the two-phase-reactor model, were optimized to maximize the yield of hydrocarbon products.
UR - http://www.scopus.com/inward/record.url?scp=84936090376&partnerID=8YFLogxK
U2 - 10.1021/acs.iecr.5b00556
DO - 10.1021/acs.iecr.5b00556
M3 - Article
AN - SCOPUS:84936090376
SN - 0888-5885
VL - 54
SP - 6749
EP - 6760
JO - Industrial & Engineering Chemistry Research
JF - Industrial & Engineering Chemistry Research
IS - 26
ER -